Simultaneous removal of soot and NOx with noble metal catalysts
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(1.Shenzhen Key Laboratory of Water Resource Utilization and Environmental Pollution Control(Harbin Institute of Technology Shenzhen Graduate School), 518055 Shenzhen, Guangdong, China; 2. Public Platform for Technological Service in Urban Waste Reuse and Energy Regeneration, 518055 Shenzhen, Guangdong, China)

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X511

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    Abstract:

    In order to systematically evaluate the activities of the noble metal catalysts for simultaneous removal of soot and NOx and the corresponding effect of sulfur and water, a series of noble metal catalysts (Ru/ZrO2, Ag/ZrO2, Rh/ZrO2, Pd/ZrO2, Pt/ZrO2, Ir/ZrO2, Au/ZrO2) were prepared by iso-volumetric impregnation method firstly. Then the activities of the noble metal catalysts for simultaneous removal of soot and NOx were measured under oxygen-rich condition, and the effect of SO2 and H2O on the performances of those catalysts were also studied. Experimental results showed that noble metal can improve the activities of simultaneous removal of soot and NOx significantly. Compared with the other catalysts, Ru/ZrO2, Ag/ZrO2and Pd/ZrO2 have higher catalytic activity. The existence of SO2 and H2O promoted Ir/ZrO2 catalystal removal of soot and NOx simultaneously, promoted Pt/ZrO2 catalyze for soot oxidation, Ru/ZrO2 for NOx reduction and inhibited the catalytic activities of other noble metals.

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History
  • Received:April 03,2014
  • Revised:
  • Adopted:
  • Online: August 06,2015
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