引用本文: | 王昭阳,齐晶瑶,王博,冯岩,李科.钢渣粒子电极三维电催化法处理模拟印染废水[J].哈尔滨工业大学学报,2015,47(8):38.DOI:10.11918/j.issn.0367-6234.2015.08.008 |
| WANG Zhaoyang,QI Jingyao,WANG Bo,FENG Yan,LI Ke.A three dimensional electrochemical oxidation reactorbased on magnetic steel slag particle electrodes for printing/dyeing wastewater treatment[J].Journal of Harbin Institute of Technology,2015,47(8):38.DOI:10.11918/j.issn.0367-6234.2015.08.008 |
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钢渣粒子电极三维电催化法处理模拟印染废水 |
王昭阳1,齐晶瑶1,王博1,冯岩1,2,李科1,3
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(1.哈尔滨工业大学 市政环境工程学院,150090 哈尔滨;2.济南大学 土木建筑学院, 250022 济南;3.吉林建筑大学 市政与环境工程学院,130118 长春)
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摘要: |
为提高钢渣的综合利用率,同时降低三维电催化技术中粒子电极的制备成本,利用钢渣制备出具有一定磁性的钢渣粒子电极.利用扫描电镜和振动样品磁强计对钢渣粒子电极的磁性与表面形貌进行了定性和定量表征,其磁饱和强度为 1.638 6 A·m2/kg.在设计好的三维电化学氧化系统中,研究其处理模拟印染废水的性能.结果表明:利用磁性钢渣粒子电极的三维电化学氧化系统降解模拟印染废水中罗丹明B的最佳条件为初始质量浓度5 mg/L,槽电压5 V,初始pH为4,支持电解质投加浓度为0.15 mol/L. |
关键词: 钢渣 磁性粒子电极 三维电化学氧化系统 罗丹明B 电芬顿作用 |
DOI:10.11918/j.issn.0367-6234.2015.08.008 |
分类号:X131.2 |
基金项目:国家自然科学基金(51178142);哈尔滨市科技创新人才研究专项基金(RC2013XK015009);山东省自然科学基金(ZR2012EEL21);山东省高等学校科技计划项目(J14LG02);山东省科技发展计划政策引导类项目立项计划(2013YD17003). |
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A three dimensional electrochemical oxidation reactorbased on magnetic steel slag particle electrodes for printing/dyeing wastewater treatment |
WANG Zhaoyang1, QI Jingyao1, WANG Bo1, FENG Yan1,2, LI Ke1,3
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(1.School of Municipal and Environmental Engineering, Harbin Institute of Technology, 150090 Harbin, China; 2. School of Civil Engineering and Architecture, University of Jinan, 250022 Jinan, China; 3. School of Municipal and Environmental Engineering, Jilin Jianzhu University, 130118 Changchun, China)
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Abstract: |
To control the production cost of the particle electrodes, a novel particle electrode was prepared using the steel slag, which has certain magnetism and could be applied for the dyeing wastewater treatment. The steel slag particle electrodes, with a saturation magnetic induction of 1.638 6 A·m2/kg, were characterized by SEM and VSM. Moreover, the prepared magnetic particle electrodes were utilized in a three-dimensional electrochemical oxidation system for simulative printing/dyeing wastewater treatment. Experimental results showed that the optimal parameters were: initial concentration of the solution of 5 mg/L, initial pH value of 4, applied voltage of 5 V, and concentration of the supporting electrolyte of 0.15 mol/L. |
Key words: steel slag magnetic particle electrodes three-dimensional electrochemical oxidation system rhodamine B electro-Fenton |